The reaction rate of a catalyzed reaction is faster than the reaction rate of the uncatalyzed reaction at the same temperature. Application In Synthesis of 2-Bromophenylacetonitrile, 19472-74-3, Name is 2-Bromophenylacetonitrile, SMILES is C1=C(C(=CC=C1)CC#N)Br, in an article , author is Watson, Geert, once mentioned of 19472-74-3.
A Ru-Complex Tethered to a N-Rich Covalent Triazine Framework for Tandem Aerobic Oxidation-Knoevenagel Condensation Reactions
Herein, a highly N-rich covalent triazine framework (CTF) is applied as support for a Ru-III complex. The bipyridine sites within the CTF provide excellent anchoring points for the [Ru(acac)(2)(CH3CN)(2)]PF6 complex. The obtained robust Ru-III@bipy-CTF material was applied for the selective tandem aerobic oxidation-Knoevenagel condensation reaction. The presented system shows a high catalytic performance (>80% conversion of alcohols to alpha, beta-unsaturated nitriles) without the use of expensive noble metals. The bipy-CTF not only acts as the catalyst support but also provides the active sites for both aerobic oxidation and Knoevenagel condensation reactions. This work highlights a new perspective for the development of highly efficient and robust heterogeneous catalysts applying CTFs for cascade catalysis.
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